Uncooled Broadband
Photodetection via Light Trapping in Conformal PtTe2–Silicon Nanopillar
Heterostructures
Posted on 2024-04-20 - 13:06
Dirac semimetals have demonstrated significant attraction
in the
field of optoelectronics due to their unique bandgap structure and
high carrier mobility. Combining them with classical semiconductor
materials to form heterojunctions enables broadband optoelectronic
conversion at room temperature. However, the low light absorption
of layered Dirac semimetals substantially limits the device’s
responsivity in the infrared band. Herein, a three-dimensional (3D)
heterostructure, composed of silicon nanopillars (SiNPs) and a conformal
PtTe2 film, is proposed and demonstrated to enhance the
photoresponsivity for uncooled broadband detection. The light trapping
effect in the 3D heterostructure efficiently promotes the interaction
between light and PtTe2, while also enhancing the light
absorption efficiency of silicon, which enables the enhancement of
the device responsivity across a broadband spectrum. Experimentally,
the PtTe2-SiNPs heterojunction device demonstrates excellent
photoelectric conversion behavior across the visible, near-infrared,
and long-wave infrared (LWIR) bands, with its responsivity demonstrating
an order-of-magnitude improvement compared to the counterparts with
planar silicon heterojunctions. Under 11 μm laser irradiation,
the noise equivalent power (NEP) can reach 1.76 nW·Hz–1/2 (@1 kHz). These findings offer a strategic approach to the design
and fabrication of high-performance broadband photodetectors based
on Dirac semimetals.
CITE THIS COLLECTION
DataCiteDataCite
No result found
Wu, Yuequan; Nie, Changbin; Sun, Feiying; Jiang, Xilong; Zhang, Xianning; Fu, Jintao; et al. (2024). Uncooled Broadband
Photodetection via Light Trapping in Conformal PtTe2–Silicon Nanopillar
Heterostructures. ACS Publications. Collection. https://doi.org/10.1021/acsami.4c00827