Ultrahighly Photosensitive and Highly Stretchable
Rippled Structure Photodetectors Based on Perovskite Nanocrystals
and Graphene
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Stretchable optoelectronic
devices are the need of the hour when it comes to making present day
technologies user-friendly. These devices when placed conformably
on the human skin or any other artificial intelligence products must
function in all their capacities to get a durable and highly sensitive
device performance. Stretchable photodetectors are the core fundamental
constituents that fall under the umbrella of flexible optoelectronic
devices. Although a significant amount of research has been reported
on stretchable photodetectors, good performance still remains a challenge.
Nanometer-sized methylammonium lead bromide ((MA)PbBr3)
perovskite nanocrystals can significantly emit and absorb light in
the visible spectrum. With high quantum yield and stable optical and
electronic properties, when they are subjected to mechanically tunable
two-dimensional (2D) composites, we obtain better performance from
stretchable optoelectronic devices. Here, a hybrid photodetector composed
of perovskite nanocrystals and graphene of rippled geometry is demonstrated,
where a thin film of photon-absorbing perovskite nanocrystals is placed
on rippled graphene that contributes to a photoresponsivity on the
order of ∼6 × 105 A W–1.
The large photoresponsivity value places this hybrid stretchable device
in the highest position among devices with similar functionality.
It is found that the photoresponsivity of the perovskite nanocrystals
and graphene hybrid rippled structure photodetector is strain tunable
with a stretchability up to 100%. In addition, the hybrid rippled
structure photodetector has wearability and durability. All of these
superior functionalities lead the way toward fabricating stretchable
optoelectronic devices suitable for applications in the fields of
biomedicine, defense systems, fire detection, and flexible display
panels.
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Chen, Ying-Huan; Kataria, Monika; Lin, Hung-I; Paul Inbaraj, Christy Roshini; Liao, Yu-Ming; Hu, Han-Wen; et al. (2019). Ultrahighly Photosensitive and Highly Stretchable
Rippled Structure Photodetectors Based on Perovskite Nanocrystals
and Graphene. ACS Publications. Collection. https://doi.org/10.1021/acsaelm.9b00308