Manganese-Catalyzed Asymmetric Oxidation of Methylene
C–H of Spirocyclic Oxindoles and Dihydroquinolinones with Hydrogen
Peroxide

Sun, Wei

Manganese-Catalyzed Asymmetric Oxidation of Methylene C–H of Spirocyclic Oxindoles and Dihydroquinolinones with Hydrogen Peroxide

Version 2 2019-01-11, 19:53

Version 1 2019-01-11, 19:48

Posted on 2019-01-11 - 19:53

A highly efficient strategy for the enantioselective oxidation of methylene C–H of spirocyclic oxindoles and dihydroquinolinones has been established, in which an earth-abundant manganese catalyst and hydrogen peroxide are used. Noteworthy, the manganese catalyst can be applied to the asymmetric hydroxylation of spirocyclic 2,3-dihydroquinolin-4-ones with 94–99% ee.

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Qiu, Bin; Xu, Daqian; Sun, Qiangsheng; Lin, Jin; Sun, Wei (2019). Manganese-Catalyzed Asymmetric Oxidation of Methylene C–H of Spirocyclic Oxindoles and Dihydroquinolinones with Hydrogen Peroxide. ACS Publications. Collection. https://doi.org/10.1021/acs.orglett.8b03652

https://doi.org/10.1021/acs.orglett.8b03652

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