Iridium-Catalyzed Enantioselective Allyl–Allyl
Cross-Coupling of Racemic Allylic Alcohols with Allylboronates
Version 2 2018-12-07, 20:12
Version 1 2018-12-03, 17:20
Posted on 2018-12-07 - 20:12
Carreira’s iridium-(P, olefin)
phosphoramidite-based catalytic
system that allows asymmetric allyl–allylboronate cross-coupling
with high enantioselectivity is reported. This transformation tolerates
a large variety of racemic branched allylic alcohols and allylboronate
substrates. The utility of the coupling is demonstrated in a concise
catalytic asymmetric synthesis of (−)-preclamol.
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Zheng, Yu; Yue, Bei-Bei; Wei, Kun; Yang, Yu-Rong (2018). Iridium-Catalyzed Enantioselective Allyl–Allyl
Cross-Coupling of Racemic Allylic Alcohols with Allylboronates. ACS Publications. Collection. https://doi.org/10.1021/acs.orglett.8b03627
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AUTHORS (4)
YZ
Yu Zheng
BY
Bei-Bei Yue
KW
Kun Wei
YY
Yu-Rong Yang