Helical
Nanographenes Embedded with Contiguous Azulene
Units
Posted on 2020-07-17 - 14:36
The
azulene moiety, composed of contiguous pentagonal and heptagonal
rings, is a structural defect that alters the electronic, magnetic,
and structural properties of graphenes and graphene nanoribbons. However,
nanographenes embedded with an azulene cluster have not been widely
investigated because these compounds are difficult to synthesize in
their pure form. Herein, azulene-embedded nanographenes bearing a
unique cove-type edge were synthesized by a novel synthetic protocol.
Experimental and theoretical investigations revealed that this cove
edge imparts stable helical chirality, unlike normal cove edges. The
in-solution self-association behavior and the structural, electronic,
and electrochemical properties were also described in detail.
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Ogawa, Naoki; Yamaoka, Yousuke; Takikawa, Hiroshi; Yamada, Ken-ichi; Takasu, Kiyosei (2020). Helical
Nanographenes Embedded with Contiguous Azulene
Units. ACS Publications. Collection. https://doi.org/10.1021/jacs.0c06156
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AUTHORS (5)
NO
Naoki Ogawa
YY
Yousuke Yamaoka
HT
Hiroshi Takikawa
KY
Ken-ichi Yamada
KT
Kiyosei Takasu