Expanding the Spectrum of Light-Driven Peroxygenase
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Version 2 2019-01-10, 20:42
Version 1 2018-12-31, 14:38
Posted on 2019-01-10 - 20:42
Peroxygenases
require a controlled supply of H2O2 to operate
efficiently. Here, we propose a photocatalytic
system for the reductive activation of ambient O2 to produce
H2O2 which uses the energy provided by visible
light more efficiently based on the combination of wavelength-complementary
photosensitizers. This approach was coupled to an enzymatic system
to make formate available as a sacrificial electron donor. The scope
and current limitations of this approach are reported and discussed.
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Willot, Sébastien
J.-P.; Fernández-Fueyo, Elena; Tieves, Florian; Pesic, Milja; Alcalde, Miguel; Arends, Isabel W.C.E.; et al. (2018). Expanding the Spectrum of Light-Driven Peroxygenase
Reactions. ACS Publications. Collection. https://doi.org/10.1021/acscatal.8b03752
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AUTHORS (8)
SW
Sébastien
J.-P. Willot
EF
Elena Fernández-Fueyo
FT
Florian Tieves
MP
Milja Pesic
MA
Miguel Alcalde
IA
Isabel W.C.E. Arends
CP
Chan Beum Park
FH
Frank Hollmann