Enhanced Hydromagnesite Process for CO2 Sequestration
by Desilication of Serpentine Ore in NaOH Solution
Posted on 2020-06-11 - 10:13
A new CO2 fixation process was highly enhanced by desilication
of serpentine ore with concentrated NaOH solution and NH3 recycling. In the process, desilicated serpentine containing up
to 83 wt % MgO after leaching is treated by NH4Cl solution,
from which MgCl2 solution and NH3 gas are generated
and are used to capture CO2. Hydromagnesite is produced
from the reaction between ammonium carbonate and MgCl2 solution
at ambient temperature. The Phase-transition diagram of magnesium
carbonate was constructed with the OLI-based chemical model. The leaching
behavior of serpentine in concentrated NaOH was systematically studied.
Parameters including the initial NaOH concentration, leaching temperature,
solid-to-liquid ratio, and reaction time were investigated to achieve
efficient separation of Si and Mg. The validity of the proposed process
is successfully verified step by step and the target product of hydromagnesite
is obtained. The synthetic hydromagnesite exhibit the same structure
and similar morphology as natural hydromagnesite. Moreover, valuable
2% Ni-bearing minerals were also produced.
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Zhang, Xiaojuan; Zeng, Yan; Li, Zhibao (2020). Enhanced Hydromagnesite Process for CO2 Sequestration
by Desilication of Serpentine Ore in NaOH Solution. ACS Publications. Collection. https://doi.org/10.1021/acs.iecr.0c01600