Enantioselective
Synthesis of Cyclobutenes by Intermolecular
[2+2] Cycloaddition with Non‑C2 Symmetric Digold Catalysts
Version 2 2017-11-09, 05:30
Version 1 2017-09-22, 17:19
Posted on 2017-11-09 - 05:30
The enantioselective intermolecular
gold(I)-catalyzed [2+2] cycloaddition
of terminal alkynes and alkenes has been achieved using non-C2-chiral Josiphos digold(I) complexes as catalysts,
by the formation of the monocationic complex. This new approach has
been applied to the enantioselective total synthesis of rumphellaone
A.
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García-Morales, Cristina; Ranieri, Beatrice; Escofet, Imma; López-Suarez, Laura; Obradors, Carla; Konovalov, Andrey I.; et al. (2017). Enantioselective
Synthesis of Cyclobutenes by Intermolecular
[2+2] Cycloaddition with Non‑C2 Symmetric Digold Catalysts. ACS Publications. Collection. https://doi.org/10.1021/jacs.7b07651
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AUTHORS (7)
CG
Cristina García-Morales
BR
Beatrice Ranieri
IE
Imma Escofet
LL
Laura López-Suarez
CO
Carla Obradors
AK
Andrey I. Konovalov
AE
Antonio M. Echavarren