es5b02635_si_001.pdf (381.21 kB)
Download fileTracking the Fate of Particle Associated Fukushima Daiichi Cesium in the Ocean off Japan
journal contribution
posted on 2015-08-18, 00:00 authored by Ken O. Buesseler, Christopher R. German, Makio
C. Honda, Shigeyoshi Otosaka, Erin E. Black, Hajime Kawakami, Steven J. Manganini, Steven M. PikeA three year time-series
of particle fluxes is presented from sediment
traps deployed at 500 and 1000 m at a site 115 km southeast of Fukushima
Daiichi Nuclear Power Plant (FDNPP). Results show a high fraction
of lithogenic material and mass flux peaks that do not align between
the trap depths, suggesting a lateral source of sediments. Fukushima
cesium-137 and cesium-134 were enhanced in flux peaks that, given
variations in trap 137Cs/210Pbex ratios,
are characteristic of material derived from shelf and slope sediments
found from <120 to >500 m. These lateral flux peaks are possibly
triggered by passing typhoons. The Cs fluxes are an order of magnitude
higher than were previously reported for the trap located 100 km due
east of FDNPP. We attribute this large difference to the position
of our trap under the southeasterly currents that carry contaminated
waters and resuspended sediments away from FDNPP and into the Pacific.
These higher Cs sedimentary fluxes offshore are still small relative
to the inventory of Cs currently buried nearshore. Consequently, we
do not expect them to effect any rapid decrease in Cs levels for the
coastal sediments near FDNPP that have been linked to enhanced Cs
in demersal fish.