posted on 2025-04-29, 13:40authored byYouxi Zhang, Ciaran Bench, Preveen Surendranathan, Mads S Bergholt
The efficiency and resolution of dispersive spectrometers
play
crucial roles in optical spectroscopy. Achieving optimal analytical
performance in optical spectroscopy requires striking a delicate balance
between employing a narrow spectrometer input slit to enhance spectral
resolution while sacrificing throughput or utilizing a wider slit
to increase throughput at the expense of resolution. Here, we introduce
a spectrometer slit empowered by a deep learning model SlitNET. We
trained a neural network to reconstruct synthetic Raman spectra with
enhanced resolution from low-resolution inputs. Subsequently, we performed
transfer learning from synthetic data to experimental Raman data of
materials. By fine-tuning the model with experimental data, we recovered
high-resolution Raman spectra. This enhancement enabled us to distinguish
between materials that were previously indistinguishable when using
a wide slit. SlitNET achieved a resolution enhancement equivalent
to employing a 10 μm slit size but with a physical input slit
of 100 μm. This, in turn, enables us to simultaneously achieve
high throughput and resolution, thereby enhancing the analytic sensitivity
and specificity in optical spectroscopy. The incorporation of deep
learning into spectrometers highlights the convergence of photonic
instrumentation and artificial intelligence, offering improved measurement
accuracy across various optical spectroscopy applications.