posted on 2021-12-13, 19:38authored byYebin Lee, Hyunwoo Choi, Haoyu Zhang, Yun Wu, Dabin Lee, William S. Wong, Xiaowu Shirley Tang, Juhyun Park, Houyong Yu, Kam C. Tam
Sensitive
strain sensors (an important component of soft robotics,
wearable devices, and biomedical electronics) with high sensitivity,
stretchability, and long-term stability are still challenging. A sensitive,
stretchable, and sustainable sensor using poly(3,4-ethylenedioxythiophene)
(PEDOT) coated cellulose nanocrystals (CNC) with poly(vinyl alcohol)/glycerol
(PVA/Gly) composite is proposed. The low cost and sustainable PEDOT
coated CNC with high aspect ratio lowered the electrical percolation
threshold that significantly improved the electrical conductivity
leading to better sensitivity (gauge factor = 21.25) compared to the
PEDOT applied film without CNC (gauge factor = 9.35). The exceptional
stretchability of up to 500% and a low Young’s modulus with
long-term stability exceeding 3 months are due to the glycerol plasticizer.
The fabricated sensors possessed outstanding real-time strain sensing
capability for a series of human motions, including complex joint
bending motions, subtle muscle motions, wrist pulse, and excellent
self-healing ability. This effective green strategy for preparing
a highly stretchable conductive composite addresses current limitations
in strain sensor preparation and offers a sustainable approach to
sensor design and development.