Observational Evidence of Large Contribution from Primary Sources for Carbon Monoxide in the South Asian Outflow

South Asian air is among the most polluted in the world, causing premature death of millions and asserting a strong perturbation of the regional climate. A central component is carbon monoxide (CO), which is a key modulator of the oxidizing capacity of the atmosphere and a potent indirect greenhouse gas. While CO concentrations are declining elsewhere, South Asia exhibits an increasing trend for unresolved reasons. In this paper, we use dual-isotope (δ¹³C and δ¹⁸O) fingerprinting of CO intercepted in the South Asian outflow to constrain the relative contributions from primary and secondary CO sources. Results show that combustion-derived primary sources dominate the wintertime continental CO fingerprint (f_primary ∼ 79 ± 4%), significantly higher than the global estimate (f_primary ∼ 55 ± 5%). Satellite-based inventory estimates match isotope-constrained f_primary-CO, suggesting observational convergence in source characterization and a prospect for model–observation reconciliation. This “ground-truthing” emphasizes the pressing need to mitigate incomplete combustion activities for climate/air quality benefits in South Asia.