posted on 2023-12-08, 19:09authored byXiaobin Zou, Ruize Wang, Mingyuan Xie, Fei Tian, Yong Sun, Chengxin Wang
Two-dimensional
(2D) materials with exotic transport behaviors
have attracted extensive interest in microelectronics and condensed
matter physics, while scaled-up 2D thin films compatible with the
efficient wet-chemical etching process represent realistic advancement
toward new-generation integrated functional devices. Here, thickness-controllable
growth and chemical patterning of high-quality Bi2O2Te continuous films are demonstrated. Noticeably, except for
an ultrahigh mobility (∼45074 cm2 V–1 s–1 at 2 K) and obvious Shubnikov–de Hass
quantum oscillations, a 2D transport channel and large linear magnetoresistance
are revealed in the patterned Bi2O2Te films.
Investigation implies that the linear magnetoresistance correlates
with the inhomogeneity described by P. B. Littlewood’s theory and EMT-RRN theory developed recently. These results
not only reveal the nonsaturating linear magnetoresistance in high-quality
Bi2O2Te but shed light on understanding the
corresponding physical origin of linear magnetoresistance in 2D high-mobility
semiconductors and providing a pathway for the potential application
in multifunctional electronic devices.