posted on 2019-07-19, 15:22authored byW. M. Brown, E. M. Gauger
We
establish design principles for light-harvesting antennae whose
energy capture scales superlinearly with system size. Controlling
the absorber dipole orientations produces sets of “guide-slide”
states that promote steady-state superabsorbing characteristics in
noisy condensed-matter nanostructures. Inspired by natural photosynthetic
complexes, we discuss the example of ringlike dipole arrangements
and show that, in our setup, vibrational relaxation enhances rather
than impedes performance. Remarkably, the superabsorption effect proves
to be robust to O(5%) disorder simultaneously for all relevant
system parameters, showing promise for experimental exploration across
a broad range of platforms.