Ionic Gel Paper with Long-Term Bendable Electrical Robustness for Use in Flexible Electroluminescent Devices

Conductive paper has low-cost, lightweight, sustainability, easy scale-up, and tailorable advantages, allowing for its promising potential in flexible electronics, such as bendable supercapacitors, solar cells, electromagnetic shields, and actuators. Ionic gels, exhibiting a lower Young’s modulus together with facile manufacturing, can fully serve as the conductive component to prepare conductive paper. Herein we report a low-cost (∼1.3 dollars/m²), continuous, and high-throughput (up to ∼30 m/min) fabrication of reliable and long-term (stable for more than two months) conductive paper. As-prepared conductive paper shows a high electrical durability with negligible bending–recovering signal changes over 5000 cycles. Using this ionic gel paper (IGP) as a key component, we build a variety of proof-of-principle demonstrations to show the capacity of IGP in constructing flexible electroluminescent devices with diverse patterns, including a square, an alphabetic string, and a laughing face. Our methodology has the potential to open a new powerful route to fabricate bendable conductive paper for a myriad of applications in future flexible electronics.