posted on 2017-03-09, 00:00authored byPragya Verma, Donald G. Truhlar
The
local approximations to exchange–correlation functionals
that are widely used in Kohn–Sham density functional theory
usually underestimate band gaps and molecular excitation energies,
and therefore, it becomes necessary to use more expensive hybrid functionals
or more empirical DFT+U functionals for accurate predictions and modeling
of these properties. This work presents a meta-generalized gradient
approximation (meta-GGA) called High Local Exchange 2017 (HLE17) and
illustrates how it can be useful for obtaining accurate semiconductor
band gaps and molecular excitation energies. Unlike the conventional
way of using the DFT+U method, one does not need to determine new
parameters for every property or system studied. The HLE17 functional
builds upon our earlier work (HLE16) where we had shown that by increasing
the coefficient of local exchange and simultaneously decreasing the
coefficient of local correlation with a GGA, the band gaps and excitation
energies could be significantly improved without significantly degrading
the ground-state molecular energetic properties. However, for almost
every database tested in this work, HLE17 shows improvement over HLE16,
and the improvement is particularly notable for solid-state lattice
constants. This new functional provides a strategy for calculating
properties that are otherwise difficult to calculate by a local functional.