posted on 2023-12-13, 14:44authored byMoritz
B. Heindl, Hua Zhu, Moungi G. Bawendi, Georg Herink
Semiconductor quantum dots offer highly flexible optoelectronic
properties, rendering them attractive for a growing number of applications,
including single-photon emitters, fluorescence microscopy, and display
technology. Here, we report the realization of an electro-absorptive
terahertz (THz) antenna based on colloidal semiconductor nanocrystals
for the phase-resolved detection of infrared lightwaves. Introducing
AC-biasing to symmetric nanocrystals, we break the symmetric response
of the quantum-confined Stark effect (QCSE) to the direction of the
THz field and obtain a polarity-sensitive observable. In particular,
we analyze the nonlinear scaling of the QCSE and demonstrate that
differential detection via bias-modulation yields a signal that linearly
depends on the THz field strength. This THz antenna employs solution-processed
quantum dots and enables an all-optical readout via absorption or
emission, offering highly flexible implementations of THz sensing
in the time domain.