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Temperature-Dependence of an Amorphous Organic Thin Film Polariton Laser
journal contribution
posted on 2020-03-27, 17:36 authored by Yue Qu, Shaocong Hou, Stephen R. ForrestSince its first observation, the
polariton lasing threshold in
organic films has been anomalously high, given that Bosonic condensation
should occur at vanishingly small pumping powers. Here, we investigate
the temperature dependence of a polariton laser employing an amorphous
organic thin film, 2,7-bis[9,9-di(4-methylphenyl)-fluoren-2-yl]-9,9-di(4-methylphenyl)fluorene,
in a vertical optical microcavity. An increase in laser threshold
is observed at temperatures <45 K, while the threshold remains
unchanged as the temperature increases up to room temperature. In
contrast, the energy dispersion characteristic of cavity polaritons
is independent of temperature. At low temperature, an energy relaxation
bottleneck along the polariton dispersion takes place below threshold.
The bottleneck is found to be responsible for the anomalous increase
in threshold with decreasing temperature. As the pumping power increases,
amplified spontaneous emission (ASE) is observed prior to the onset
of lasing. We also study the photoluminescence of the neat organic
film versus temperature to explain the origin of the bottleneck in
the exciton polariton dispersion.
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temperature dependencepolariton lasing thresholdfilmtemperature increasesexciton polariton dispersionASElaser thresholdpower increasesAmorphous Organicpolariton dispersionenergy relaxation bottleneckFilm Polariton Laserpolariton lasercavity polaritonsenergy dispersionroom temperatureBosonic condensation
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