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Characteristics of Fine Particulate Matter and Polycyclic Aromatic Hydrocarbons Emitted from Coal Combustion Processes
journal contribution
posted on 2019-09-19, 13:45 authored by Chia Ming Lu, Nguyen Duy Dat, Chian Kou Lien, Kai Hsien Chi, Moo Been ChangCharacteristics and
emission factors of condensable particulate
matter (CPM) and filterable particulate matter (FPM2.5)
and polycyclic aromatic hydrocarbons (PAHs) (16 U.S. EPA PAHs and
15 + 1 EU PAHs) emitted from a coal-fired power plant (plant A) and
a coal-fired boiler (plant B) in Taiwan were investigated via stack
samplings. Removal efficiencies of CPM, FPM2.5, and PAHs
achieved with baghouse (BH) + seawater flue gas desulfurization (SWFGD)
were also evaluated for plant A. Results indicate that CPM concentrations
measured in plants A and B are 12.7 ± 1.44 and 28.0 ± 6.32
mg/Nm3, respectively, which are significantly higher than
FPM2.5 concentrations measured in two plants. The CMP/FPM
ratios measured in plants A and B are 12.7 ± 1.44 and 28.0 ±
6.32, respectively. The organic content is the major contributor to
CPM collected from plant A (90 ± 3.7%), while the inorganic content
contributes 93 ± 2.4% of CPM collected from plant B. Furthermore,
different compositions of soluble ion are found in CPM/FPM collected
from the stacks of plants A and B. This difference might be attributed
to different coal used, varying combustion efficiencies, and different
removal efficiencies of organic and inorganic contents achieved with
different air pollution control devices (APCDs) with different operating
temperatures in plants A and B. The average PAH concentrations measured
at stacks of plants A and B are 28.4 and 43.4 μg/Nm3, respectively. Gaseous PAHs predominate in terms of both mass and
toxic equivalency (TEQ) concentrations, acounting for 99.5 and 96.0%,
respectively. The 15 + 1 EU PAHs contribute 99.0 and 99.99% to total
TEQ of gaseous and particulate PAHs, respectively. The removal efficiency
of CPM achieved with BH and SWFGD of plant A is 38.3%, which is significantly
lower than that of FPM2.5 (99.8%) and PM (99.9%). The PAH
removal efficiency achieved with APCDs in plant A increases as the
ring number increases. The overall PAH removal efficiencies achieved
with the APCDs of plant A are 89.8 and 94.3% based on mass and TEQ
concentrations, respectively.
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CPMBHCoal Combustion Processes CharacteristicsEPASWFGDseawater flue gas desulfurizationremoval efficienciesFPM 2.5PAH removal efficienciesair pollution control devicesplant BCMPFine Particulate MatterTEQring number increases1 EU PAHsU.SAPCDPAH removal efficiencyFPM 2.5 concentrationsPolycyclic Aromatic Hydrocarbons Emitted
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